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Synthesis and characterization of novel 3′-N-deacylated, 16alpha-hydroxy-15-methyl-pregnenolone.
16alpha-Hydroxy-15-methyl-pregnenolone (16alpha-OH-15-Me-P) was first synthesized from progesterone (6beta-acetoxy-16alpha-hydroxy-5beta-pregnane-3,20-dione) using regioselective enzymatic deacetylation. The epimerization of 16alpha-OH-15-Me-P to 16alpha-OH-15-epimer-15-Me-P was achieved using a regioselective epimerization method. In both cases the N-deacylated steroids showed an additional 3′-COOH group and were purified using reverse phase C-18 and adsorption chromatography on a YMC column. The dehydrogenated steroids were further separated using reverse phase adsorption chromatography. The spectral data and IR and 1H-NMR spectrum of 16alpha-OH-15-Me-P showed that the hydrogen in the C-3 position was replaced by a hydroxyl group. The formation of the C-20 hydroxy group was confirmed by the extensive hydrogen-deuterium exchange and/or 2D NMR spectroscopic studies. The dehydrogenated steroids were characterized by mass spectrometry, 1H-NMR, 13C-NMR and high resolution mass spectrometry.[Frequency of medical diagnosis and medical treatment of migraine in Germany].
To determine the frequency of migraine as a diagnostic and a therapeutic clinical entity in Germany, the prevalence of migraine sufferers in the population of Germany was established by using four different sampling methods: during three years (1978 to 1980) a representative epidemiological study was performed in a sample of 38,000 subjects from a primary care setting by a multistage sampling method; during two years (1982 to 1983) in a random sample of 1,563 representative patients with migraine and without headache
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